Biophysics and Other Topics by Aharon Katzir-Katchalsky

By Aharon Katzir-Katchalsky

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Die Feldenergie von Polyelektrolytmolekulen wurde iherniodynaiiiisch mittels potentiometrischer Titration bestimmt. Es wurde gezeigt, dass sie vom Molekulargewicht, von der Polymerkonzentration und von der Ionenstarke abhangt. Es wurde gefunden, dass die Ladung der Feldenergie pro ionisierte Gruppe vom Molekulargewicht unabhangig ist. Die elektrostatische Feldenergie wurde theoretisch aus statistischen und elektrostatischen Betrachtungen berechnet, und mittels Benutzung eines vereinfachteu Models wurde eine angenaherte Formel erhalten.

T h e constancy of thermodynamic potential may be compared with temperature constancy and hence the isopotential step may be compared with the isothermals of thermodynamics. In order t o maintain equilibrium with the bath, the restrictive condition o f the relation between the number o f ionized groups and the molecular extension is given b y equations (9) and (24). T h e increase in h causes a decrease in the molecular field energy and makes the dissociation o f protons from acidic groups easier.

69, 192 (1950). 5. , and Kimball, G. , J. , 5, 115 (1950). 6. Kuhn, W . , Helv. Chim. Acta, 31, 1994 (1948). 7. Katchalsky, A . , and Kuhn, W . , J. Polymer ScL, 5, 283 (1950). 8. Katchalsky, A . , J. Polymer ScL, 6, 145 (1951). 9. Fuoss, R . M . , J. , 3, 603 (1948). 10. Fuoss, R . M . , and Cathers, G. , J. Polymer ScL, 4, 97 (1949). 11. Fuoss, R . M . , and Strauss, U. , Ann. N. Y. Acad. , 51, 836 (1949). 12. , unpublished results. 13. D o b r y , A . , J. chim. , 47, 402 (1950). 14. , Fitzgerald, N .

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